Towards a closed loop recycling process of end-of-life lithium-ion batteries: Recovery of critical metals and electrochemical performance evaluation of a regenerated LiCoO2

The growing demand for lithium-ion battery technology emphasizes the critical need to establish effective recycling and proper disposal methods for used batteries, ensuring the long-term sustainability and security of the battery supply chain. This study addresses this need by exploring two hydrochemical routes, using sulfuric acid and nitric acid, respectively. The objective is to investigate the influence of the acid used in the leaching process on the properties of the regenerated final product, LiCoO2. Moreover, a novel and simplified approach for extracting lithium as lithium carbonate is proposed.