Modelling of a hybrid bioelectrocatalytic flow reactor with NADH cofactor regeneration by immobilized rhodium mediator for pyruvate bioconversion

Wassim El Housseini,Mathieu Etienne,Elisabeth Lojou,Alain Walcarius,François Lapicque

Chemical Engineering and Processing - Process Intensification（2023）

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摘要

•A hybrid bioelectrochemical flow reactor for pyruvate bioreduction has been modelled.•Rh-mediated NADH regeneration and LDH-catalysed reduction occur on stacked layers.•Mass transfer rate to Rh(I) are intensified by the stacked LDH-immobilized CNT-layer.•Redox reduction of NAD+ by Rh(I) is no more first-order wrt. NAD+ in dilute solutions.

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关键词

Flow reactors,Bioelectrocatalytic processes,NADH regeneration,Rh complex,Lactate dehydrogenase catalysis,Pyruvate bioconversion

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