Synergistic effect of surface Cu0 and Cu+ species on improved selective hydrogenation of furfural to furfuryl alcohol over hydrotalcite-derived CuxMg3Al oxides

Applied Surface Science（2023）

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摘要

•Preparation of CuxMg3AlOy mixed-metal oxides derived from CuMgAl-LDHs.•High activity of furfural to furfuryl alcohol over CuxMg3AlOy without H2 pre-treatment.•Surface CuOx species can be reduced in situ to Cu0 species during the reaction.•Cu0 and Cu+ contribute to H2 activation and adsorption of furfural, respectively.•Synergistic effect of surface Cu0 and Cu+ species on promoting hydrogenation reaction.

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关键词

Cu x Mg 3 AlO y oxides, Cu 0 species, Cu plus species, Synergistic effect, Selective hydrogenation of furfural, Furfuryl alcohol

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