Unique Li deposition behavior in Li3PS4 solid electrolyte observed via operando X-ray computed tomography

Jaehee Park,Toshiki Watanabe,Kentaro Yamamoto,Tomoki Uchiyama,Tsuyoshi Takami,Atsushi Sakuda,Akitoshi Hayashi,Masahiro Tatsumisago,Yoshiharu Uchimoto

CHEMICAL COMMUNICATIONS（2023）

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摘要

The problem of lithium dendrites must be addressed for practical lithium metal all-solid-state batteries. Herein, three-dimensional morphological changes within Li3PS4 electrolyte away from the anode were observed using operando X-ray computed tomography. We revealed that the electronic conduction of decomposition and the electrolyte/void interface cause the lithium deposition within the Li3PS4.

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unique li deposition behavior,solid electrolyte,x-ray

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