Activation of Alkyl Chlorides Enabled by Zirconocene and Photoredox Catalysis
crossref(2022)
摘要
C–Cl bond cleavage of unactivated alkyl chlorides with zirconocene and photoredox catalysis has been achieved. The present protocol exhibited a broader scope of alkyl chlorides compared to the preceding methods with titanocene. This scope expansion could be attribut-ed to the zirconium metal center rendering the C–Cl bond cleavage more endergonic and lowering the transition states.
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