From Femtosecond Excited-State and Dissociation Dynamics to Nanosecond Reaction Kinetics: Following C-H Bond Activation with X-rays

Raphael M. Jay,Ambar Banerjee,Torsten Leitner,Robert Stefanuik,Ru-Pan Wang, Jessica Harich,Emma Beale,Victoria Kabanova,Abdullah Kahraman,Anna Wach, Dimitri Ozerov, Christopher A. Arrell,Philip J. M. Johnson,Grigory Smolentsev,Thomas Huthwelker, Camilia N. Borca,Claudio Cirelli,Camila Bacellar,Christopher J. Milne,Nils Huse,Michael Odelius,Philippe Wernet

The International Conference on Ultrafast Phenomena (UP) 2022（2022）

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摘要

Using ultrafast X-ray absorption spectroscopy, we observe how a rhodium carbonyl catalyst is formed on femtosecond timescales and reveal the decisive orbital interactions which facilitate the efficient cleavage of an alkane C-H bond from solution.

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nanosecond reaction kinetics,dissociation dynamics,excited-state,x-rays

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