Fluorine-free MXene activate peroxymonosulfate to remove tetracyclic antibiotics

Feng Wang,Zhaoyong Bian,Wenhai Zhang,Lei Zheng,Yaru Zhang,Hui Wang

Separation and Purification Technology（2023）

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摘要

•Fluorine-free-Ti3C2Tx was prepared using tetramethylammonium hydroxide.•Ff-Ti3C2Tx/PMS system exhibited dramatic catalytic activity for TC degradation.•The contributions of 1O2 and ·O2− to TC were 45.3% and 30.2%, respectively.•Pathway and toxicity of TC intermediates in Ff-Ti3C2Tx/PMS system were revealed.

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关键词

Ti3C2Tx MXene,Fluorine-free,Peroxymonosulfate,Tetracyclic antibiotics,Degradation mechanism

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