Structure and performance sensitivity to simulated An4+ waste doping in a high-silicon glasses-ceramics

Yang He,Xiaoyan Shu,Mingfen Wen,Guilin Wei,Yuexiang Lu,Yi Xie,Faqin Dong,Shunzhang Chen,Kuibao Zhang,Xiaoan Li,Xirui Lu

Materials Science and Engineering: B（2023）

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摘要

•CeO2 improved the O/Si to drive glass network rearrangement.•Some Ce4+ are reduced under the influence of magnetite and CeO2 crystal defects.•Most Ce ions are hidden in a frame-like network of aluminosilicate glass.•The loading limit to CeO2 is broken by adjusting Al/Si in granite.

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关键词

Novel immobilization matrix,Pyroreaction,Immobilization mechanism,Structure and Performance,Charge compensator

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