Manganese(III) complexes with tetradentate O^C^C^O ligands: Synthesis, characterization and catalytic studies on the CO2 cycloaddition with epoxides

Giammarco Meloni, Luca Beghetto,Marco Baron,Andrea Biffis,Paolo Sgarbossa,Miriam Mba,Paolo Centomo,Laura Orian,Claudia Graiff,Cristina Tubaro

Molecular Catalysis（2023）

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摘要

•Optimized synthesis of tetradentate bis(NHC)-bis(phenolate) ligands.•First example of hexacoordinated Mn(III) complex with NHC ligands.•Synthesis of cyclic carbonates from CO2 and epoxides.•CO2 chemical valorization through a catalytic approach.

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关键词

Homogeneous catalysis,CO2 chemical valorization,Phenolate ligands,Manganese organometallics,N-heterocyclic carbene

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