Ligands hydrophobicity dependent electrocatalytic CO2 reduction activities of Sn5-oxo clusters

Fang-Fang Liu,Di Wang,Guang-Hui Chen,Jian Zhang,Lei Zhang

Journal of Solid State Chemistry（2023）

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摘要

Two Sn5-oxo clusters with isostructural cores, (nBuSn)5(μ3-O)2(EG4)L3 (H2EG = ethylene glycol, L = 4-tert-butylbenzoate or 4-hydroxybenzoate), have been successfully prepared using (nBuSn)OH2Cl as tin source precursor. Comparative studies of contact angle test and electrocatalytic carbon dioxide reduction reveal that the 4-tert-butylbenzoate decorated Sn5 with more hydrophobic surface possesses higher catalytic activity.

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关键词

Tin-oxo clusters,Ligands effect,Contact angle,Electrocatalytic CO2 reduction

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