Turning photocatalytic H2 evolution into CO2 reduction of molecular nickel(II) complexes by using a redox–active bipyridine ligand

Ting Liu,Youting Fang,Yang Li,Yukang Fu,Duobin Chao

Journal of Molecular Structure（2023）

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摘要

•Two Ni(II) complexes with redox-active and redox-innocent ligands are designed and synthesized.•Both photocatalytic CO2 reduction and H2 evolution were studied for the two Ni(II) complexes.•The Ni(II) complex containing a redox-active ligand can catalyze photoreduction of CO2.•The Ni(II) complex without a redox-active ligand is more suitable for photocatalytic H2 evolution.

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关键词

Photocatalysis,CO2 reduction,H2 evolution,Nickel complex,Redox–active ligand

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