Towards frustration in Eu(II) Archimedean tessellations.

Hua Chen,Anna S Manvell,Mariusz Kubus,Maja A Dunstan,Giulia Lorusso,David Gracia, Mike S B Jørgensen,Søren Kegnæs,Fabrice Wilhelm,Andrei Rogalev,Marco Evangelisti,Kasper S Pedersen

Chemical communications (Cambridge, England)（2023）

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摘要

Self-assembly of -{EuI} nodes and ditopic ligands leads to isoreticular 2D frameworks featuring a rare, non-kagome Archimedean tessellation. The topology and intra-layer Eu(II)-Eu(II) antiferromagnetic interactions provide the prerequisites for geometrical spin frustration, which, due to the spin state degeneracy, is key for novel phenomena such as enhanced magnetic refrigeration.

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