Mechanism of Sulfur Poisoning to Ru-Based Catalysts in Supercritical Water Gasification of Glycerol: From Experiment to Combined Dft and Kinetics Studies

Xinyu Cui,Haoran He, Dan Xie,Lixiao Zheng,Xuebin Wang, Zhao Jiang,Donghai Xu,Yang Guo

SSRN Electronic Journal（2023）

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摘要

•Deactivation of Ru-based catalysts induced by sulfur poisoning is investigated.•Reveal the competitive adsorption between CO and sulfur after catalyst poisoning by DFT calculations.•A kinetic model is developed based on a possible network for SCWG of glycerol with sulfur presence.

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关键词

supercritical water gasification,glycerol,sulfur poisoning,catalysts,ru-based

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