Rational Integration of Carbon Nanotubes into Chain‐Engineered Bipolar Polyimides as Core‐Shell Heterostructured Electrodes for Polymer‐Based Symmetrical Full Batteries (Adv. Funct. Mater. 5/2023)

Bipolar Polymer Full-Batery In article number 2211590, Yingkui Yang and co-workers fabricate robust hierarchical core-shell heterostructures by combining polyquinone imines with carbon nanotubes. Such highly redox-active composites overcome the proverbial barriers of organic electrodes in terms of poor rate capability, low active site utilization, and lower cycling stability, enabling their use as bipolar electrodes for building sustainable full batteries with high energy and power density.