Cross sections and calculated yields of some radionuclides of yttrium, strontium and rubidium formed in proton-induced reactions on enriched strontium-86: possibility of production of Sr-85g, Rb-83 and Rb-82m in no-carrier-added form

RADIOCHIMICA ACTA(2023)

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摘要
Cross sections of the Sr-86(p,3n)Y-84m, Sr-86(p,alpha n)Rb-82m, and Sr-86(p,x)Sr-85g reactions were measured from their respective thresholds up to 16.2 MeV and from 23.0 to 44.1 MeV at FZJ, and from 14.3 to 24.5 MeV at LBNL, using 96.4% enriched (SrCO3)-Sr-86 as target material. Thin targets prepared by sedimentation were irradiated with protons in a stacked-form, and the induced radioactivity was measured by high-resolution gamma-ray spectrometry. Nuclear model calculations based on the code TALYS reproduced our experimental cross section data well. From the excitation functions, the integral yields of the above three radionuclides were calculated. The yield of Sr-85g via the Sr-nat(n,gamma) process was also measured using the TRIGA Mark-II reactor at AERE, Savar. A comparison of the reactor and cyclotron production of carrier-added Sr-85g is given. The production possibilities of the three investigated radionuclides in no-carrier-added forms at a 30 MeV cyclotron via new routes are discussed.
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(SrCO3)-Sr-86 thin samples, cyclotrons and TRIGA Mark II reactor, excitation function, integral yield and isotopic purity of the product, nuclear model calculation, proton- and neutron-irradiations
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