Defect engineering and post-synthetic reduction of Cu based metal–organic frameworks towards efficient adsorption desulfurization

Canyang Zhang,Xiaowei Zhang,Zhiping Tao,Baozhen Li,Danfeng Zhao,Hongyi Gao,Zhongpeng Zhu,Ge Wang,Xingtian Shu

Chemical Engineering Journal（2022）

引用 11|浏览7

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摘要

•ADS performance of the best CuBDC-x is 104.5% higher than the original CuBDC.•Both the defects and porosity can be regulated by a defect engineering method.•A convenient ethanol thermal treatment is developed to reduce Cu2+ to Cu+.•Cu+ rather than Cu2+ are demonstrated to be the adsorption site of mercaptan.

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关键词

Adsorption desulfurization,Mercaptan,Defect,Cu2+ reduction,Metal organic framework

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