Construction of lithophilic solid electrolyte interfaces with a bottom-up nucleation barrier difference for low-N/P ratio Li-metal batteries

Jinlong Jiang,Xiaofeng Hu,Shangying Lu,Chao Shen,Shoushuang Huang,Xiaoyu Liu,Yong Jiang,Jiujun Zhang,Bing Zhao

Energy Storage Materials（2022）

引用 14|浏览9

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摘要

•A LiF/LixMgy layer is prepared on Au/Cu foil to obtain nucleation barrier difference.•Li is guided to deposit preferentially between the LiF/LixMgy and Au layer.•DFT calculation results demonstrate the fast Li+ kinetics of LiF-rich layer.•The full cell presents stable cycling at low N/P ratio and lean electrolyte content.

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关键词

LiF/LixMgy artificial layer,Solid electrolyte interphase,Nucleation barrier difference,Young's modulus,Li metal anode

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