Redox potential regulated by electrolyte concentration: A case study of electrochemical oxidation of 2,2,6,6-tetramethyl piperidine-1-oxyl

Feng Zhu, Yuhan Zou, Liwen Hua, Xiaolian Peng, Wenbin Zhang

Electrochemistry Communications（2022）

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摘要

•The redox potential of TEMPO can be regulated by electrolyte concentration.•The diffusion coefficients of TEMPO decrease as the concentration of LiTFSI increases.•The redox potential of TEMPO shifts negatively with an increase in LiTFSI concentration.•Solvation energy changes and ion pairing are the main contributors to these effects.

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关键词

TEMPO,Supporting electrolyte,Potential shift,Solvation effect,Ion pairing

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