Can CO2 be a catalyst? Yes, CO2-catalyzed N-formylation of aliphatic amines with DMF

Xiao-Chao Chen,Lin Guo,Guang-Hui Shi,Kai-Chun Zhao,Yong Lu,Ye Liu

Molecular Catalysis（2022）

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摘要

•CO2 serving as an efficient and clean catalyst.•CO2-catalyzed N-formylation of aliphatic amines with DMF.•Characterization of the carbamate salt as a catalyst-substrate (CO2-alphatic amine) adduct.

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关键词

CO2 catalyst,N-formylation,Formylating reagents,in situ high-pressure FT-IR spectra,Carbamate salt

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