Impact of speciation on the tellurium electrochemistry in choline chloride-based deep eutectic solvents

Alassane Sorgho,Moussa Bougouma,Gael De Leener,Julien Vander Steen,Thomas Doneux

Electrochemistry Communications（2022）

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摘要

•• Speciation of Te(IV) differs in two choline chloride-based deep eutectic solvents.•• [TeCl6]2− is kinetically labile and leads to a fast reversible electrochemistry.•• In choline chloride-urea, hydrolysis produces oxo-chloro Te(IV) complexes.•• Oxo-chloro species are kinetically inert leading to non-reversible electrochemistry.

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关键词

pH of deep eutectic solvents,Lability of tellurium complexes,125Te NMR,Rotating disc electrode

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