Guanidine-embedded poly(ionic liquid) as a versatile precursor for self-templated synthesis of nitrogen-doped carbons: Tailoring the microstructure for enhanced CO2 capture

Chong Chen,Yukun Zhang,Qiuhao Li,Yunlong Wang,Jun Ma

Fuel（2022）

引用 7|浏览2

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摘要

•Guanidine-embedded poly(ionic liquid) (PTMG) was synthesized by terpolymerization.•N-doped carbon materials CTMGs were constructed by pyrolysis and activation.•Self-decomposition of PTMG precursor favored the formation of ultra-micropores.•In-situ generated pyrrolic-N sites strengthened the binding force toward CO2.•Desirable CO2 uptake, CO2/N2 selectivity and cyclic performance was attained.

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关键词

Guanidine-based poly(ionic liquid),Self-templated synthesis,Nitrogen-doped carbon,Ultra-microporous,CO2 capture

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