Simulation and Testing of the Radiation Performance of SiC Particles with Different Distribution Morphologies

PHOTONICS(2022)

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摘要
Based on Mie scattering theory, fractal theory, the generalized multiparticle Mie model and the attenuated total reflectance infrared spectroscopy method, this paper aimed to explore the influence of different distribution morphologies of semiconductor nanoparticles on their radiation properties. The results revealed that (1) the symmetry and fluctuation amplitude of the scattering direction of the SiC elementary particles, with a diameter of 100 nm, and the cluster particles were related to the wavelength, particle size and agglomeration state. (2) The particle size distribution had a significant effect on the spectral extinction performance of the SiC particles, especially when lambda > 10 mu m, which can be greatly strengthened by increasing the proportion of large-scale particles. (3) The influence of SiC particle clusters on their spectral extinction was directly related to the cluster size and wavelength. When lambda < 10 mu m, small-scale cluster particles showed lower extinction performances; however, the absorption and scattering factors increased with the increase in cluster size while lambda > 10 mu m, and the extinction performance significantly improved. In summary, the quantitative changes in the microscale and structure, as well as the distribution states, had a significant impact on the infrared spectral characteristics of the particles, and we expect to adjust the particle size distribution to obtain desired radiation properties.
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关键词
elementary particles, cluster particles, particle agglomeration, particle scattering, Mie scattering theory, generalized multiparticle Mie theory, fractal theory, attenuated total reflectance infrared spectroscopy method
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