High Performance Carbon Dioxide Electroreduction in Ionic Liquids with in Situ Shell-Isolated Nanoparticle-Enhanced Raman Spectroscopy

Ye Hu,Zhongdong Gan,Shixian Xin,Wenhui Fang,Yanlei Wang,Wei Cui,Hong Zhao,Zengxi Li,Xiangping Zhang

SSRN Electronic Journal（2022）

引用 8|浏览8

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摘要

•The electrochemical reduction of CO2 was studied in imidazolium ionic liquids.•The maximum CO Faraday efficiency of 94.6% in BmimCl/MeCN was obtained.•The current density was 72 mA cm−2 at −2.2 V vs Ag/Ag+.•The intermediates CO2·– and CO32– were observed by in situ Raman spectra.

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关键词

Electrochemical CO2 reduction,Ionic liquids,Raman spectroscopy,Shell-isolated nanoparticles

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