Reduction of HgCl2 to Hg0 in flue gas at high temperature. Part Ⅰ: Influences of oxidative species

Tianfang Huang, Xinze Geng,Xiaoshuo Liu, Jiang Liu,Yufeng Duan, Shilin Zhao,Rajender Gupta

Fuel（2022）

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摘要

•The quartz filler with appropriate size can promote the HTD of HgCl2(g).•The presence of active Cl atoms is a crucial factor hindering the HTD of HgCl2(g).•Cl atoms and O can promote the generation of HgO with intermediates ClO, which is a vital transition product for Hg0 re-oxidation.•A rapid cooling process can avoid the hazard of Hg0(g) re-oxidation by chlorine species.

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关键词

Hg-CEMS,High-temperature decomposition,HgCl2(g) reduction,Hg0(g) re-oxidation,Oxidative species

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