Ultrafast excited state relaxation dynamics in a heteroleptic Ir(iii ) complex, fac-Ir(ppy)2(ppz), revealed by femtosecond X-ray transient absorption spectroscopy
Inorganic Chemistry Frontiers（2021）
摘要
The experimental and calculation results demonstrate that the 3MLppzCT state generated by the spin-forbidden transition rapidly relaxes to 3MLppyCT through internal conversion process with a time constant of ∼450 fs.
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