Low temperature structures and magnetic interactions in the organic-based ferromagnetic and metamagnetic polymorphs of decamethylferrocenium 7,7,8,8-tetracyano-p-quinodimethanide, [FeCp*₂]˙⁺[TCNQ]˙⁻

Saul H. Lapidus,Peter W. Stephens,Maria Fumanal,Jordi Ribas-Ariño,Juan J. Novoa,Jack G. DaSilva,Arnold L. Rheingold,Joel S. Miller

Dalton Transactions（2021）

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摘要

To identify the genesis of the differing magnetic behaviors for the ferro- (FO) and metamagnetic (MM) polymorphs of [FeCp*2][TCNQ] the low temperature structures of each polymorph were determined from high-resolution synchrotron powder diffraction data.

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Low temperature structures and magnetic interactions in the organic-based ferromagnetic and metamagnetic polymorphs of decamethylferrocenium 7,7,8,8-tetracyano-p-quinodimethanide, [FeCp*2]˙+[TCNQ]˙−

Low temperature structures and magnetic interactions in the organic-based ferromagnetic and metamagnetic polymorphs of decamethylferrocenium 7,7,8,8-tetracyano-p-quinodimethanide, [FeCp*₂]˙⁺[TCNQ]˙⁻