Probing the generality of spin crossover complex T_½vs. ligand ¹⁵N NMR chemical shift correlations: towards predictable tuning

Luca Bondì,Santiago Rodríguez-Jiménez,Humphrey L. C. Feltham,Anna L. Garden,Sally Brooker

Inorganic Chemistry Frontiers（2021）

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摘要

A study of 6 families (42 members) demonstrates that within a family the easily calculated 15N-NMR values of ligands enable predictable tuning of T1/2 in the corresponding complexes, except for 2 families with weakly influencing meta-substituents.

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Probing the generality of spin crossover complex T½vs. ligand 15N NMR chemical shift correlations: towards predictable tuning

Probing the generality of spin crossover complex T_½vs. ligand ¹⁵N NMR chemical shift correlations: towards predictable tuning