CO oxidation on MgAl₂O₄ supported Ir_n: activation of lattice oxygen in the subnanometer regime and emergence of nuclearity-activity volcano

Yubing Lu,Coogan Thompson,Chun-Te Kuo,Xiwen Zhang,Adam S. Hoffman,Alexey Boubnov,Simon R. Bare,Libor Kovarik,Hongliang Xin,Ayman M. Karim

Journal of Materials Chemistry A（2022）

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摘要

Ir subnanometer clusters activate surface oxygen on a traditionally non-reducible MgAl2O4 support which leads to a more active two-site mechanism during low-temperature CO oxidation.

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CO oxidation on MgAl2O4 supported Irn: activation of lattice oxygen in the subnanometer regime and emergence of nuclearity-activity volcano

CO oxidation on MgAl₂O₄ supported Ir_n: activation of lattice oxygen in the subnanometer regime and emergence of nuclearity-activity volcano