Selectivity and efficiency of nitrite electroreduction catalyzed by a series of Keggin polyoxometalates

Yulin Zhou, Francois Bihl,Antoine Bonnefont,Corinne Boudon,Laurent Ruhlmann,Vasilica Badets

Journal of Catalysis（2022）

引用 7|浏览5

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摘要

•Redox behavior POMs determine the onset potential of nitrite electroreduction.•Microkinetic model allows simulation of experimental data and calculation of TOF.•The rate constant of POMs catalyzed nitrite electroreduction is dependent on the pH.

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关键词

DEMS,Keggin type polyoxometalate,Nitrite reduction,Nitrous acid reduction,Nitrous oxide,Nitric oxide,Turnover frequency,Microkinetic model

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