Enhancing CH4/N2 separation performance within aluminum-based Metal-Organic Frameworks: Influence of the pore structure and linker polarity

Zhenghui Huang,Peng Hu,Jia Liu,Fang Shen,Youquan Zhang,Kungang Chai,Yunpan Ying,Chengjun Kang,Zhaoqiang Zhang,Hongbing Ji

Separation and Purification Technology（2022）

引用 21|浏览7

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摘要

•Al-MOFs show satisfying but varying CH4/N2 selectivity due to tunable pore structure.•Linker polarity affecting CH4 affinity was also verified via simulations.•AlO6 availability and polar surface synergistically promoted CH4 uptake.•Above two merits rendered Al-Fum a promising adsorbent for CH4/N2 separation.

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关键词

Adsorption,Al-fumarate,CH4/N2 separation,Metal–organic framework,Theoretical simulation

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