Measuring gamma doses over the mGy-kGy range with a single type of TLD detector

Adrien Gruel,Alix Sardet, Vincent Chaussonnet, Maxime Houdouin-Quenault, Daniel Garnier

ANIMMA 2021 - ADVANCEMENTS IN NUCLEAR INSTRUMENTATION MEASUREMENT METHODS AND THEIR APPLICATIONS(2021)

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摘要
Thermo-luminescent detectors are currently used to measure gamma doses in the medical and environmental surveillance fields. During the past few years, the CEA Reactor Studies Division tested and validated the use of these detectors for gamma flux characterization and nuclear heating measurements in mixed neutron/gamma fields of low power reactors. Doses were comprised between a few mGy and a few Gy for dose rates up to a few Gy.h(-1). However, in MTR or TRIGA reactors, the gamma flux level is much higher (> 10(12) n/cm(2)/s) and the TLD currently in use (CaF2:Mn and (LiF)-Li-7:Mg,Ti) and their readout protocols were no longer suitable for the resulting doses. In order to extend the applicable dose range up to similar to 1 MGy (dose rate of a few kGy.h(-1)), several options were explored. On one side, some adjustments were made to the readout protocols of CaF2:Mn and (LiF)-Li-7:Mg,Ti, notably by testing the use of filters to reduce the amount of light received by the reader PMT to avoid saturation. On the other side, a new type of TLD (LiF:Mg,Cu,P) with different Li enrichments (natural or enriched in Li-7) was tested. This paper presents the calibration measurements results performed in pure gamma fields, at the irradiation platform of the CEA Cadarache Radioprotection Division, between 250 mGy and 3 Gy for all detector types. In addition to the calibration, these measurements also studied the Mg,Cu,P-doped detectors response: reproducibility, dose rate dependence, incoming photon energy dependence, high temperature effect when reading TLD, etc. Results show that at low doses Mg,Cu,P-doped TLDs are slightly less stable than CaF2:Mn and (LiF)-Li-7:Mg,Ti. The sensitivity modification after a high dose exposure seems to indicate that a new protocol readout should be defined for Mg,Cu,P-doped sensors (high temperature peak).
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关键词
TLD, calibration, gamma dose
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