Magnetic properties of 1D spin systems with compositional disorder of three-spin structural units

ZEITSCHRIFT FUR NATURFORSCHUNG SECTION B-A JOURNAL OF CHEMICAL SCIENCES(2021)

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摘要
The exact diagonalization (ED) approach and Quantum Monte-Carlo (QMC) method were used for the study of the lowest energy states and low-temperature magnetic properties of some disordered 1D Heisenberg spin-1/2 systems formed by two types of three-spin structural units. For the system with a singlet ground state and the random distribution of structural units along the chain system, a significant decrease of the size of the intermediate magnetization plateau in comparison to the corresponding uniform spin system was found. For the "polyallyl" spin chain with a macroscopic value of the ground state spin, a transition to the singlet ground state due to the effect of compositional disorder was observed.
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关键词
compositional disorder, Heisenbergspin-1/2 chains, intermediate magnetization plateau, Quantum Monte-Carlo method (QMC), the energy spectrum
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