Support Effect and Surface Reconstruction in In2O3/m-ZrO(2)Catalyzed CO2 Hydrogenation br

Xueqiang Zhang, Alexey Kirilin,Steve Rozeveld,Joo H. Kang,Glenn Pollefeyt,David F. Yancey,Adam Chojecki,Britt Vanchura,Monika Blum

ACS Catalysis（2022）

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摘要

We investigate the chemical and structural dynamics at the interface ofIn2O3/m-ZrO2and their consequences on the CO2hydrogenation reaction(CO2HR) under reaction conditions. While acting to enrich CO2, monocliniczirconia (m-ZrO2) was also found to serve as a chemical and structural modifier ofIn2O3that directly governs the outcome of the CO2HR. These modifying effectsinclude the following: (1) Under reaction conditions (above 623 K), partiallyreduced In2O3, i.e., InOx(0 更多

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关键词

In2O3, m-ZrO2, support effect, in situ, CO2&nbsp, hydrogenation, reconstruction, ambient pressure X-ray photoelectron spectroscopy

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