Encapsulating UiO-66-NH2@Pt with defective PCN-222 as an active armor to fabricate a sandwich-type nanocatalyst for the tandem synthesis via hydrogenation of nitroarenes

Hong Li,Yiming Wang,Rongxiu Guo,Jianwei Zheng,Zejun Sun,Xinyue Zhang,Ying Guo,Hongna Jia,Qionglin Liang,Hong-bin Sun

Journal of Catalysis（2022）

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摘要

•UiO-66-NH2@Pt@PCN-222 as a multifunctional catalyst.•Encapsulating UiO-66-NH2@Pt with defective PCN-222 as an active armor.•A cascade reaction to form β-ketoenamines via the hydrogenation of nitroarenes.•The matched rate of the successive reactions benefits the selectivity for a cascade.

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关键词

Sandwich-nanostructure catalyst,Metal organic frameworks,MOFs encapsulation,Tandem synthesis,β-ketoenamines,Hydrogenation of nitroarenes,Atmospheric H2

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