Tracking the Fe^IV(O) intermediate and O–O bond formation of a nonheme iron catalyst for water oxidation

Bing Yang,Qing-Qing Yang,Xin Jiang,Bin Chen,Chen-Ho Tung,Li-Zhu Wu

Chemical Communications（2017）

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摘要

We describe here a new complex 1 by subtle modulation of the TPA ligand and succeed in capturing the high-valent FeIV(O) species, which is responsible for the O–O bond formation and oxygen evolution with higher efficiency.

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Tracking the FeIV(O) intermediate and O–O bond formation of a nonheme iron catalyst for water oxidation

Tracking the Fe^IV(O) intermediate and O–O bond formation of a nonheme iron catalyst for water oxidation