Catalytic hydrogenation of CO2 with unsymmetric N-heterocyclic carbene-nitrogen-phosphine ruthenium complexes

Li Ji,Tianhua Cui,Xufeng Nie,Yanling Zheng,Xueli Zheng,Haiyan Fu,Maolin Yuan,Hua Chen,Jiaqi Xu,Ruixiang Li

Catalysis Science & Technology（2021）

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摘要

Unsymmetric Ru-CNP and Ru-CN(H)P complexes are synthesized and applied in the hydrogenation of CO2 to formate for the first time. The Ru-CNP complex shows excellent stability and high activity. The TON is around 170 000 after 48 h at 200 degrees C, which is a relatively high record value among all the Ru complexes.

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