Evidence of dynamical effects and critical field in a cobalt spin crossover complex

Thilini K Ekanayaka,Ping Wang,Saeed Yazdani,Jared Paul Phillips,Esha Mishra,Ashley S Dale,Alpha T N'Diaye,Christoph Klewe,Padraic Shafer,John Freeland,Robert Streubel,James Paris Wampler,Vivien Zapf,Ruihua Cheng,Michael Shatruk,Peter A Dowben

CHEMICAL COMMUNICATIONS（2022）

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摘要

The [Co(SQ)(2)(4-CN-py)(2)] complex exhibits dynamical effects over a wide range of temperature. The orbital moment, determined by X-ray magnetic circular dichroism (XMCD) with decreasing applied magnetic field, indicates a nonzero critical field for net alignment of magnetic moments, an effect not seen with the spin moment of [Co(SQ)(2)(4-CN-py)(2)].

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