Transcription-induced formation of paired Al sites in high-silica CHA-type zeolite framework using Al-rich amorphous aluminosilicate

Mizuho Yabushita,Yoshiyasu Imanishi,Ting Xiao,Ryota Osuga,Toshiki Nishitoba,Sachiko Maki,Kiyoshi Kanie,Wenbin Cao,Toshiyuki Yokoi,Atsushi Muramatsu

CHEMICAL COMMUNICATIONS（2021）

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摘要

The paired Al species pre-formed in Al-rich amorphous aluminosilicates were transcribed into high-silica CHA-type zeolite frameworks under hydrothermal conditions, which offers a new approach to creating paired Al sites in zeolite frameworks. This Al-pair-rich CHA exhibited a higher Sr2+ uptake than the control CHA zeolite synthesized by the conventional procedure.

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