Structural, dielectric and reflection analysis of ZnxMg1-xTiO3 ceramics synthesized using auto-ignition combustion method

JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS(2021)

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摘要
Zinc-substituted magnesium titanate ZnxMg1-xTiO3 (x = 0.00-0.10, delta x = 0.025) solid solutions were synthesized using auto-ignition combustion process and characterized for structural, dielectric and reflection properties. X-ray diffraction analysis discovered the creation of single-phase MgTiO3. Scanning electron microscopy (SEM) indicated the existence of low porosity closely packed grains. The study of the dielectric properties indicated that for ZnxMg1-xTiO3 with x = 0.05, a reasonably great combination of the relative permittivity (e(r)) with value 16.60, loss tangent (tan delta) of 0.9 x 10(-3) and temperature coefficient of resonant frequency (tau(f)) of - 41.37 ppm/degrees C at 10 kHz was observed. The electromagnetic reflection analysis at microwave frequencies (12.4-26.5 GHz) revealed that composition x = 0.05 shows maximum 90% reflection bandwidth of 5.60 GHz in the Ku frequency band and 4.59 GHz in the K frequency band. These materials with low to intermediate relative permittivity, low losses, and a minor negative temperature coefficient of resonant frequency might be utilized as a resonator, antenna, and filter substrate for next-generation communication devices.
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关键词
ceramics,dielectric,auto-ignition
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