A Facile Strategy to Achieve Large Triplet Gap Based on Excited-State Aromaticity-tunable Five-memebered Ring
ChemRxiv(2021)
摘要
We have proposed a facile strategy
to achieve large triple gap by manipulating the aromaticity and the transition
properties of the low-lying excited states, then theoretically designed and
experimentally verified a series of donor-bridge-acceptor based on partially
conjugated five-membered rings with high aromaticity in T1 state to meet the
harsh energy conditions required for hot
exciton materials and for singlet fission materials.
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