A sustainable and green route to furan-2,5-dicarboxylic acid by direct carboxylation of 2-furoic acid and CO2

Yu-Gao Wang,Chong-Yang Guo,Jun Shen,Yu-Qin Sun,Yan-Xia Niu,Peng Li,Gang Liu,Xian-Yong Wei

Journal of CO2 Utilization（2021）

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摘要

•Carboxylation involved hydrogen abstraction in 2-furoate and electrophilic addition of CO2.•Hydrogen abstraction of furan ring was rate-determining.•Selective generation of 2,5-FDCA depended on hydrogen abstraction step and molecular features of 2-furoate.

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关键词

Chemical utilization of CO2,Synthesis of 2,5-furandicarboxylic acid,Direct carboxylation,Lignocellulose bio-based compound

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