An Alginate-Confined Peroxygenase-Clea For Styrene Epoxidation

Friederike E H Nintzel,Yinqi Wu,Matteo Planchestainer,Martin Held,Miguel Alcalde,Frank Hollmann

CHEMICAL COMMUNICATIONS（2021）

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摘要

Oxyfunctionalisation reactions in neat substrate still pose a challenge for biocatalysis. Here, we report an alginate-confined peroxygenase-CLEA to catalyse the enantioselective epoxidation of cis-beta-methylstyrene in a solvent-free reaction system achieving turnover numbers of 96 000 for the biocatalyst and epoxide concentrations of 48 mM.

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