Atomic nickel cluster decorated defect-rich copper for enhanced C2 product selectivity in electrocatalytic CO2 reduction

Xiaolong Zhang,Chuangwei Liu,Yong Zhao,Linbo Li,Yu Chen,Fazal Raziq,Liang Qiao,Si-Xuan Guo,Caiyun Wang,Gordon G. Wallace,Alan M. Bond,Jie Zhang

APPLIED CATALYSIS B-ENVIRONMENTAL（2021）

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摘要

•A coordination enabled galvanic replacement method was developed.•This method was used to decorate defect-rich copper with atomic nickel clusters.•The catalyst was used for electrochemical reduction of CO2.•Multi-carbon product selectivity was significantly enhanced.•The reaction mechanism was revealed by detailed DFT calculations.

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关键词

Carbon dioxide reduction, Electrocatalysis, Bimetallic catalyst, Surface decoration

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