Evidences for the random singlet phase in a new honeycomb iridate SrIr$_2$O$_6$

arxiv(2021)

引用 0|浏览4
暂无评分
摘要
Strong spin-orbital-coupling magnetic systems with the honeycomb structure can provide bond-directional interactions, which may result in Kitaev quantum spin liquids and exotic anyonic excitations. However, one of the key ingredients in real materials -- disorders -- has been much less studied in Kitaev systems. Here we synthesized a new trigonal SrIr$_2$O$_6$, which consists of two-dimensional honeycomb Ir planes with edge-sharing IrO$_6$ octahedra. First-principle computation and experimental measurements suggest that the electronic system is gapped and there should be no magnetic moment as the Ir$^{5+}$ ion has no unpaired electrons. However, significant magnetism has been observed in the material and it can be attributed to disorders that are most likely from oxygen vacancies. No magnetic order is found down to 0.05 K and the low-temperature magnetic properties exhibit power-law behaviors in magnetic susceptibility and zero-field specific heat, and a single-parameter scaling of the specific heat under magnetic fields. These results provide strong evidences for the existence of the random singlet phase in SrIr$_2$O$_6$, which offers a new member to the family of spin-orbital coupled iridates and Kitaev materials.
更多
查看译文
关键词
random singlet phase,new honeycomb
AI 理解论文
溯源树
样例
生成溯源树,研究论文发展脉络
Chat Paper
正在生成论文摘要