A cubane-type manganese complex with H2O oxidation capabilities

Swetanshu Tandon,Joaquin Soriano-Lopez,Amal C. Kathalikkattil,Guanghua Jin,Paul Wix,Munuswamy Venkatesan,Ross Lundy,Michael A. Morris,Graeme W. Watson,Wolfgang Schmitt

SUSTAINABLE ENERGY & FUELS（2020）

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摘要

We report the synthesis and characterisation of [Mn8K2O4(OH)(2)((CH3)(3)CCOO)(16)(CH3CN)(2)] whose cluster core shares some features with the oxygen evolving complex (OEC), the natural water oxidation catalyst. Importantly, this complex provides a bio-inspired complex that promotes catalytic H2O oxidation at neutral pH value.

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