Ultrafast bi-excitonic dynamics and annihilation in molecular and mesoscopic systems

Pavel Malevich,Constantin Heshmatpour,Craig N. Lincoln,Harald Ceymann,Maximilian H. Schreck,Juergen Hauer

EPJ Web of Conferences（2019）

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摘要

We present 5th and 3rd order 2D spectra of a squarine trimer. Slowly decaying (tau = 0.8 ps) and intensity dependent features unique to the 5th order signal are attributed to exciton-exciton annihilation.

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