Polariton-assisted emission of strongly coupled organic dye excitons in a tunable optical microcavity

Proceedings of SPIE(2019)

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摘要
Light-matter coupling between the molecular dipole transitions and a confined electromagnetic field provides the ability to control the fundamental properties of coupled matter. The use of tunable optical microcavities for electromagnetic field confinement allows one to affect the coupled state properties in a controllable manner, whereas the coupling strength in this system strongly depends on the transition dipole moment and a mode volume of the cavity. In this study we have demonstrated controllable emission of Rhodamine 6G organic molecules with relatively low and unoriented dipole moments in a strong coupling regime by placing them into a tunable Fabry-Perot microcavity.
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关键词
light-matter interaction,tunable microcavity,polariton emission,strong coupling,Rhodamine 6G,Rabi splitting,exciton-polariton
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