Janus Evaporators With Self-Recovering Hydrophobicity For Salt-Rejecting Interfacial Solar Desalination
ACS NANO(2020)
摘要
The recent advancements in interfacial evaporation of salty water using renewable solar energy provide one of the promising pathways to solve worldwide water scarcity. Pursuing a stable evaporation rate of water has been the central focus of this field, as it is directly related to the throughput, while salt deposition on the evaporator becomes a critical issue. Although Janus-structured evaporators with an upper hydrophobic layer and a bottom hydrophilic layer have been demonstrated as an effective way to suppress the salt precipitation, the hydrophobic upper layer, achieved usually by some special organic groups, suffers from a photochemical oxidation when exposed to oxidative chemicals in water and high-energy light, resulting in a deteriorated surface hydrophobicity. Here, we report our design of an efficient salt-rejecting Janus evaporator by taking advantage of the self-recovering surface hydrophobicity of poly(dimethylsiloxane) (PDMS) against photochemical damages, which ensures a long-term surface hydrophobicity. With its upper layer partially covered with PDMS, the Janus evaporator demonstrates an excellent salt rejection capability and exhibits a stable evaporation rate of 1.38 kg.m(-2).h(-1) under 1 sun illumination for 400 min of continuous operation, or 90 d of intermittent work. By combining the advantages of high structural integration, long-term salt-rejection, and efficient evaporation, our Janus evaporator holds great promise for the stable production of clean water from seawater.
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关键词
steam generation, solar thermal, self-recovering hydrophobicity, interfid cial evaporation, salt resistance
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