Singlet Fission in Self-assembled Amphipathic Tetracene Nanoparticles: Probing the Role of Charge-transfer State

Xinyu Yan,Heyuan Liu,Xiangyang Wang,Shanshan Liu,Dezhi Zhao,Zhaofeng Tang,Jun Zhou,Xiyou Li

Journal of Photochemistry and Photobiology A: Chemistry（2020）

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摘要

•Two nanoparticles of amphipathic tetracene with different PEG lengths have been prepared with simple re-precipitation method.•Singlet fission can be conducted in these two nanoparticles via a real charge-transfer intermediate state.•Longer PEG chain will lead a reduced interaction in nanoparticle and thus a lower singlet fission yield.

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关键词

singlet fission,charge-transfer state,tetracene,colloidal nanoparticle

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