The interference fringes of above-threshold ionization spectrum of SF(6)molecules in an IR plus XUV laser field

JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS(2020)

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摘要
The interference fringes of above-threshold ionization (ATI) spectrum from atoms or molecules have been extensively studied. In this paper, we investigate the ATI of the polyatomic molecule SF(6)in IR + XUV two-color laser fields, and find that some interference fringes on the spectrum are from the molecular structure, which is independent of the parameters of the laser field. Based on the frequency-domain theory, we analyze the interference fringes for different orbitals of SF(6)molecules in detail. It is found that the orbital of SF(6)can be simplified by several terms in the region of high value of momentum, where the destructive interference fringes from these terms may carry the information of the molecular structure. Furthermore, we obtain destructive interference formulas from these simplified orbitals, which may predict the interference fringes on the ATI spectrum. Additionally, we may obtain the information about the bond length of molecules. It will be useful for the study of the ionization spectrum of polyatomic molecules.
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关键词
interference fringes,above-threshold ionization spectrum,IR plus XUV laser field,SF(6)molecule
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